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The Michigan–Ontario Ozone Source Experiment (MOOSE) is an international air quality field study that took place at the US–Canada Border region in the ozone seasons of 2021 and 2022. MOOSE addressed binational air quality issues stemming from lake breeze phenomena and transboundary transport, as well as local emissions in southeast Michigan and southern Ontario. State-of-the-art scientific techniques applied during MOOSE included the use of multiple advanced mobile laboratories equipped with real-time instrumentation; high-resolution meteorological and air quality models at regional, urban, and neighborhood scales; daily real-time meteorological and air quality forecasts; ground-based and airborne remote sensing; instrumented Unmanned Aerial Vehicles (UAVs); isotopic measurements of reactive nitrogen species; chemical fingerprinting; and fine-scale inverse modeling of emission sources. Major results include characterization of southeast Michigan as VOC-limited for local ozone formation; discovery of significant and unaccounted formaldehyde emissions from industrial sources; quantification of methane emissions from landfills and leaking natural gas pipelines; evaluation of solvent emission impacts on local and regional ozone; characterization of the sources of reactive nitrogen and PM2.5; and improvements to modeling practices for meteorological, receptor, and chemical transport models.